Using a brass wire wheel on a drill works good as your first step.
I don't mean to be contrary for sport James, but I don't agree. I made that mistake when I was doing my 400, and most of the "brass" wire wheels are in fact brass coated steel. The ones that ARE all brass fall apart instantly.
It is all-too-easy to put deep scratches in soft aluminum with rotary brushes as I learned, and then you created more, harder work to remediate them.
What's being left unsaid is blasting. If the engine is apart, they a homemade or Harbor Freight soda blaster will do a dandy job of cleaning and removing clearcoat, followed by hand abrasives and polish.
I'm in the camp of NEVER blasting with anything harder than baking soda on an engine that isn't totally disassembled, and even then, I have seen glass beads come to grief on an engine that was disassembled. But that's a whole 'nuther line of discussion.