Actually, carb sync doesn't have much effect on vibration at higher throttle openings, such as at cruising speed, a least at the typical variation you are likely to see. If you are getting excessive vibration now that you weren't getting before, it is likely to be something else. Check all the motor mounts for tightness. Check the exhaust mounting on the engine and chassis, as well. Check the rest of the bike's fasteners while you are at it.
Has the bike been down at all, even something minor as falling off the stand?
Greg
'75 CB750F