I don't believe there is any need for larger jets. There is certainly not enough info so far to make such a determination.
And, the present configuration of the bike is such a minor deviation from stock that jetting changes are unwarranted, imo.
Certainly clean the emulsion tubes.
Choke terminology:
Choke butterflies closed, equals choke "ON". For the 022A carbs, (which is what a 1975 Cb550K model would have had leaving the showroom) choke on is lever up position for this condition.
The choke increases throat pressure differential, which forces more fuel from all jets while blocking air intake.
After warm up, no choke should be need, and the lever should be fully down. After warm up is also when the idle speed is adjusted via the big idle screw. Book idle value is 1100 RPM. Note that when the engine is cold, the idle stop will be at an RPM too low for the engine to run, and must be kept up with throttle grip. After warm up, the engine will again idle on it's own at 1100 RPM.
The 022a carbs have slide adjusters for each slide position. The drill bit method frequently gets people in trouble, as it allows all the adjusters to be skewed where the slide can't physically close regardless of idle knob position. While the carbs are off, make sure at least one carb can reach all the way to the carb "floor". Lock that adjustment off, and then use that carb as a master carb to adjust the others to equal.
This applies to both bench and vacuum sync.
Ignore the numbers on vacuum sync gauges. Do ensure the manometers can read equal from a common source. Then adjust each carb to equal the reading on the master carb, and you are done with the sync. You must have all the choke butterflies open = choke off, as those butterfly plates can effect what each carb allows for vacuum reading.
Do you still have the original pilot jets (#38)? Did you examine the replacement jet emulsion tubes with respect to hole size, number of holes, tube length, and placement along the tube?
If the pilot jet is non-stock, you may need a different air screw setting. I usually set this for throttle response under load for the lowest setting that gives me good engine pick up while in any gear, including 5th, with a throttle input of 1/2 total throttle travel. This makes the idle mixture over rich, but, not enough to create a fouling build up on the spark plugs.
FYI, I had a no name 4 into 2 system on my 74 CB550 for 15 years before a swapped back to the 4 into 4 system. No carb changes were ever needed for that exhaust change.
I would never change the main jet unless a plug deposit reading or a dyno fuel map report told me that was necessary.
Cheers,